Twin wire arc is a commonly used thermal spray technology for application of steel coatings to cast iron components. Hardness and adhesion strength are critical properties of such coatings; and significant research is available reporting these properties. However; residual stresses and the anisotropic structure of the coatings leads to significantly different behavior in bending applications than in the purely tensile loading of the standard adhesion test. In addition; microstructural features that are controlled by certain process parameters during deposition of the coating can have a significant effect on these properties. This work seeks to relate the hardness and pull-off adhesion strength to the coating microstructure; and to assess the related bending strength and failure mode. Comparisons between bend tests and pull-off adhesion tests show significant differences to consider when evaluating twin wire arc coatings.